Upgrading to a dual core CPU would get a few more FPS. I got about 10 more on newer games when I went from a 3700+ to a FX-60 on the same PC. Upgrading your vidoe card will make the most differene though. I would go with a 8800GT or 9000 series. That way you could keep you motherboard.
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Asus A8N-Deluxe w/ AMD FX-60
2 GB (4x512MB) OCZ DDR400
eVGA 880GTS 640MB
600 watt PSU
2 x 74GB WD Raptor 10K on RAID 0
Windows XP Pro SP2
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