I have a similar setup to you, with the CNPS9500LED, Arctic Silver 5 and an Opteron 144 overclocked to 2.42Ghz. My load temperature is 51 degrees, so I shouldn't worry too much.
Spreading AS5 over the surface before applying the cooler will make little difference, and may increase the chances of air pockets. The best way to apply is as Arctic Silver recommends, putting a dollop in the center and letting pressure spread it for you.
My load temp is with the fan speed on minimum, so wasisnt may be onto something there as well.
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